基于单料烟的加热卷烟与传统卷烟香气成分释放差异分析
Differential analysis in aroma component release between heated cigarettes and traditional cigarettes based on unblended leaf tobacco
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摘要: 将10种单料烟分别制备成加热卷烟和传统卷烟两种类型卷烟样品,采用GC-MS分析和正交偏最小二乘法判别分析(OPLS-DA)模型评价加热卷烟气溶胶和传统卷烟主流烟气中香气成分的释放差异。结果表明:加热卷烟气溶胶和传统卷烟主流烟气中分别鉴定出53种和77种香气成分;两者共有香气成分47种,其中13种香气成分在加热卷烟气溶胶中的释放量较为突出,除乙酸、γ-丁内酯外,其他11种均是醛酮类化合物;筛选出两种卷烟中存在显著释放差异的香气成分53种,包含吡嗪吡啶类7种、酮类12种、呋喃类4种、酸类9种、酯类3种、酚类8种、烃类9种、醇类1种,从差异性香气成分在该类别总鉴定成分的占比来看,酚类香气成分在两种卷烟中的释放差异性最为显著,其余依次为烃类、吡嗪吡啶类、酸类、酯类、酮类、呋喃类、醇类。
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关键词:
- 单料烟 /
- 加热卷烟 /
- 传统卷烟 /
- 香气成分 /
- 正交偏最小二乘法判别分析
Abstract: To explore the differences between the release of aroma components in the heated cigarette and the traditional cigarette, 10 unblended leaf tobacco were prepared into two types of cigarettes. The aroma components in the aerosol of heated cigarettes and in the mainstream smoke of traditional cigarette were analyzed by GC/MS. And orthogonal partial least squares discriminant analysis (OPLS-DA) model were used to evaluate the differences of aroma components in the two types of cigarettes. The results showed that a total of 53 and 77 aroma components were identified in the aerosol of heated cigarettes and in the mainstream smoke of traditional cigarettes, respectively. Among the 47 common components, the release of 13 aroma components in the heated cigarettes were more than traditional cigarettes, such as, acetic acid, γ-Butyrolactone and the other 11 aldehyde ketone compounds. 53 different aroma components between heated cigarettes and traditional cigarettes were screened by OPLS-DA, including 7 pyrazine-pyridines,12 ketones, 4 furans, 9 acids, 3 esters, 8 phenols, 9 hydrocarbons, and 1 alcohol. According to the proportion of differential aroma components in the total identified components of the same category, the most significant differences in the release of phenolic components were observed between the two types of cigarettes, followed by hydrocarbons, pyrazine-pyridines, acids, esters, ketones, furans, alcohols. -
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[1]
刘亚丽,王金棒,郑新章,等.加热不燃烧烟草制品发展现状及展望[J].中国烟草学报,2018,24(4):91-106.
-
[2]
吴君章,沈光林,孔浩辉,等.不同单料烟叶主流烟气气溶胶粒度分布差异[J].中国烟草学报,2015(2):10-18.
-
[3]
刘嘉莉,建辉,庹苏行,等. HS-SPME-GC/MS法测定主流烟气中8种香味成分的逐口释放量[J].烟草科技,2016(1):31-37,71.
-
[4]
阎瑾,鲍峰伟,牛丽娜,等.吹扫捕集-气相色谱/质谱测定烟支挥发性成分[J].烟草科技,2020,53(4):50-58.
-
[5]
李登科,田楠,田志章,等.应用顶空气相-离子迁移谱与相对气味活度值法分析卷烟特征香气物质[J].分析测试学报,2021,40(8):1164-1170.
-
[6]
邓其馨,苏明亮,黄延俊,等.不同滤嘴通风中细支卷烟烟气主要中性和碱性香味成分逐口释放规律[J].中国烟草学报,2022,28(1):17-26.
-
[7]
楚文娟,王宏伟,田海英,等.圆周及滤嘴通风对卷烟主流烟气碱性香味成分释放量的影响[J].烟草科技, 2020,53(2):34-41.
-
[8]
纪旭东,何山,赵赛月,等.不同风格类型卷烟碱性香味成分差异化研究[J].西南农业学报,2020,33(3):651-657.
-
[9]
曹建敏,别瑞,王玉华,等.烤烟新品种中烟特香301特征香气物质研究[J].中国烟草科学,2022,43(2):64-70.
-
[10]
吴秉宇,费婷,罗辰,等.细支卷烟不同加香方式香味成分的转移行为[J].烟草科技,2021,54(1):24-31.
-
[11]
古君平,陶红,汪军霞,等.卷烟滤嘴设计对爆珠单体香料成分释放行为的影响[J].烟草科技, 2021, 54(1):32-45.
-
[12]
刘钻福,窦玉青,张本强,等.烘烤工艺对加热卷烟烤烟原料香气成分及感官质量的影响[J].中国烟草科学,2022,43(3):57-63.
-
[13]
罗彦波,陈小静,李翔宇,等.化学衍生-液相色谱-串联质谱法测定加热卷烟烟气中的醛酮类香味成分[J].分析化学,2020,48(6):794-801.
-
[14]
司晓喜,向本富,蒋薇,等.加热卷烟气溶胶中香气成分的GC-MS/MS同时测定和比较[J].食品与机械, 2021,37(6):86-96.
-
[15]
陈芝飞,陈泽少,罗灿选,等.加热卷烟气溶胶中6种酯类单体香料转移行为研究[J].轻工学报,2022,37(3):58-64.
-
[16]
邓其馨,陈辉,林艳,等.温度对加热卷烟酸性成分释放的影响[J].烟草科技,2022,55(8):49-56.
-
[17]
王颖,杨文彬,王冲,等.加热不燃烧卷烟产品主流烟气中香味成分的比较[J].食品与机械,2019,35(6):64-68.
-
[18]
杨继,汤建国,尚善斋,等.利用顶空-GC/MS法对比新型卷烟和传统卷烟的挥发性成分[J].烟草科技, 2015,48(11):33-39.
-
[19]
刘天择,杨菁,汪旭,等.不同部位烤烟化学成分及热解产物与加热卷烟感官质量的关系[J].中国烟草科学,2023,44(1):77-84.
-
[20]
中华人民共和国国家质量监督检验检疫总局,中国国家标准化管理委员会.烟草及烟草制品调节和测试的大气环境:GB/T 16447-2004[S].北京:中国标准出版社,2004.
-
[21]
罗昌荣,张乾,印黔黔,等.多步逐级裂解技术研究卷烟燃时香味成分形成与温度之间的关系[J].食品与生物技术学报,2022,41(12):96-104.
-
[22]
JAMES M,LIU C,CHRISTOPHER P,et al. Assessment of tobacco heating product THP1. 0[J]. Regulatory Toxicology and Pharmacology,2018,93:14-33.
-
[23]
董文霞.裂解气相色谱-质谱法在烟草分析中的应用研究[D].杭州:浙江工业大学,2014.
-
[24]
VICKI B,RAMESH S,DONALD M,et al. Physical characterization of pyrolyzed tobacco and tobacco components[J]. Journal of Analytical and Applied Pyrolysis,2003,66(1/2):191-215.
-
[25]
MCGRATH T E, BROWN A P, MERUVA N K, et al. Phenolic compound formation from the low temperature pyrolysis of tobacco[J]. Journal of Analytical and Applied Pyrolysis,2009,84(2):170-178.
-
[26]
朱浩,柴国璧,迟广俊,等.卷烟主流烟气烟熏香成分的感官导向分析[J].烟草科技,2017,50(1):41-49.
-
[27]
周慧明,华青,陶立奇,等.加热非燃烧状态下再造烟叶颗粒香味成分的释放行为[J].烟草科技,2019,52(5):67-76.
-
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