JOURNAL OF LIGHT INDUSTRY

CN 41-1437/TS  ISSN 2096-1553

×
“关于规范使用生成式人工智能工具的启事

菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能

罗钰湲 ,  李辛娅 ,  梁佳翔 ,  刘泓漾 ,  代笛菲 ,  郭小玲 ,  戴宏杰

downloadPDF
罗钰湲, 李辛娅, 梁佳翔, 等. 菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能[J]. 轻工学报, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
引用本文: 罗钰湲, 李辛娅, 梁佳翔, 等. 菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能[J]. 轻工学报, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
shu
LUO Yuyuan, LI Xinya, LIANG Jiaxiang, et al. Preparation and dye adsorption properties of pineapple peel cellulose/bentonite composite hydrogels[J]. Journal of Light Industry, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
Citation: LUO Yuyuan, LI Xinya, LIANG Jiaxiang, et al. Preparation and dye adsorption properties of pineapple peel cellulose/bentonite composite hydrogels[J]. Journal of Light Industry, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
shu

菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能

  • 1. 西南大学 食品科学学院, 重庆 400715;

  • 2. 重庆市朝阳中学, 重庆 400700

    • 作者简介: 罗钰湲(1999-),女,重庆市人,西南大学硕士研究生,主要研究方向为纤维素及蛋白食品胶体。E-mail:854261043@qq.com;

  • 基金项目: 重庆市雏鹰计划项目(CY210202)
    国家自然科学基金项目(31901683)
    重庆市自然科学基金项目(cstc2020jcyj-msxmX0087)

  • 中图分类号: TS209

Preparation and dye adsorption properties of pineapple peel cellulose/bentonite composite hydrogels

  • 1. College of Food Science, Southwest University, Chongqing 400715, China;

  • 2. Chongqing Chaoyang Middle School, Chongqing 400700, China

  • Received Date: 2022-03-05

    CLC number: TS209

  • 摘要: 以菠萝皮渣纤维素(PPC)为原料,通过碱/尿素体系溶解纤维素并掺入皂土,利用化学交联和原位嵌入磁性Fe3O4制备复合水凝胶,并对其结构和染料吸附性能进行研究。结果表明:皂土和Fe3O4在复合水凝胶中成功嵌入,皂土有效改善了水凝胶的交联多孔网络结构、热稳定性和溶胀性能。此外,添加皂土有利于提高水凝胶对亚甲基蓝的吸附性能,其饱和吸附量从28.09 mg/g提高到55.87 mg/g;吸附过程符合准二级动力学模型和Langmuir模型,属于化学吸附和单分子层吸附过程。
    Abstract: The pineapple peel cellulose(PPC) was used as raw material to dissolve in an alkali/urea solution with incorporation of bentonite, then further chemically cross-linked and in-situ embedded with magnetic Fe3O4 to form composite hydrogels. The structure and dye adsorption properties of hydrogels were studied. The results confirmed the successful intercalation of bentonite and Fe3O4 in the hydrogels. The bentonite effectively improved the cross-linked porous network structure, thermal stability and swelling properties of the hydrogel. The bentonite also enhanced the methylene blue adsorption performance of the hydrogels, showing an increased saturated adsorption capacity from 28.09 mg/g to 55.87 mg/g. The adsorption process conformed to the pseudo-second-order kinetic model and Langmuir model, belonging to chemical adsorption and monolayer adsorption.
    1. [1]

      赵大洲.改性香蕉皮对废水中Pb2+的循环吸附性能研究[J].轻工学报,2018,33(4):37-41.

    2. [2]

      王光荣,高世霞,于晓锋,等.改性玉米芯对Zn2+和Cu2+的吸附性能研究[J].轻工学报,2019,34(2):56-62.

    3. [3]

      DAI H J,HUANG Y,ZHANG H,et al.Direct fabrication of hierarchically processed pineapple peel hydrogels for efficient Congo red adsorption[J].Carbohydrate Polymers,2020,230:115599.

    4. [4]

      DAI H J,OU S Y,HUANG Y,et al.Utilization of pineapple peel for production of nanocellulose and film application[J].Cellulose,2018,25(3):1743-1756.

    5. [5]

      DAI H J,HUANG H H.Enhanced swelling and responsive properties of pineapple peel carboxymethyl cellulose-g-poly (acrylic acid-co-acrylamide) superabsorbent hydrogel by the introduction of carclazyte[J].Journal of Agricultural and Food Chemistry,2017,65(3):565-574.

    6. [6]

      行云逸,黄惠华.菠萝果肉纤维素水凝胶的制备及对益生菌的包埋与缓释分析[J].食品科学,2021,42(1):8-14.

    7. [7]

      关莹,陈阁谷,张冰,等.农林生物质材料基水凝胶的研究进展[J].林产化学与工业,2015,35(2):171-178.

    8. [8]

      HAMIDON T S,ADNAN R,HAAFIZ M K,et al.Cellulose-based beads for the adsorptive removal of wastewater effluents:A review[J].Environmental Chemistry Letters,2022,20(3):1965-2017.

    9. [9]

      DAI H J,HUANG H H.Modified pineapple peel cellulose hydrogels embedded with sepia ink for effective removal of methylene blue[J].Carbohydrate Polymers,2016,148:1-10.

    10. [10]

      DAI H J,HUANG Y,HUANG H H.Eco-friendly polyvinyl alcohol/carboxymethyl cellulose hydrogels reinforced with graphene oxide and bentonite for enhanced adsorption of methylene blue[J].Carbohydrate Polymers,2018,185:1-11.

    11. [11]

      宁可心,张婷,王毅,等.黏土类吸附剂去除水中污染物的研究进展[J].化工新型材料,2020,48(8):276-280.

    12. [12]

      SANTOSO S P,KURNIAWAN A,SOETAREDJO F E,et al.Eco-friendly cellulose-bentonite porous composite hydrogels for adsorptive removal of azo dye and soilless culture[J].Cellulose,2019,26(5):3339-3358.

    13. [13]

      WANG M Z,LI Y H,CUI M F,et al.Barium alginate as a skeleton coating graphene oxide and bentonite-derived composites:Excellent adsorbent based on predictive design for the enhanced adsorption of methylene blue[J].Journal of Colloid and Interface Science,2022,611:629-643.

    14. [14]

      DAI H J,HUANG Y,ZHANG Y H,et al.Green and facile fabrication of pineapple peel cellulose/magnetic diatomite hydrogels in ionic liquid for methylene blue adsorption[J].Cellulose,2019,26(6):3825-3844.

    15. [15]

      ZHANG H,LUAN Q,TANG H,et al.Removal of methyl orange from aqueous solutions by adsorption on cellulose hydrogel assisted with Fe2O3 nanoparticles[J].Cellulose,2016,24(2):903-914.

    16. [16]

      KAMEL S,EL-GENDY A A,HASSAN M A,et al.Carboxymethyl cellulose-hydrogel embedded with modified magnetite nanoparticles and porous carbon:Effective environmental adsorbent[J].Carbohydrate Polymers,2020,242:116402.

    17. [17]

      JIANG M W,NIU N,CHEN L G.A template synthesized strategy on bentonite-doped lignin hydrogel spheres for organic dyes removal[J].Separation and Purification Technology,2022,285:120376.

    18. [18]

      SANTOSO S P,ANGKAWIJAYA A E,BUNDJAJA V,et al.Investigation of the influence of crosslinking activation methods on the physicochemical and Cu (Ⅱ) adsorption characteristics of cellulose hydrogels[J].Journal of Environmental Chemical Engineering,2022,10(1):106971.

    19. [19]

      MOHAMED R R,ABU ELELLA M H,SABAA M W,et al.Synthesis of an efficient adsorbent hydrogel based on biodegradable polymers for removing crystal violet dye from aqueous solution[J].Cellulose,2018,25(11):6513-6529.

    20. [20]

      ALAM M N,ISLAM M S,CHRISTOPHER L P.Sustainable production of cellulose-based hydrogels with superb absorbing potential in physiological saline[J].ACS Omega,2019,4(5):9419-9426.

    21. [21]

      SANTIAGO F,MUCIENTES A E,OSORIO M,et al.Preparation of composites and nanocomposites based on bentonite and poly (sodium acrylate).Effect of amount of bentonite on the swelling behaviour[J].European Polymer Journal,2007,43(1):1-9.

    22. [22]

      DATTA CHAUDHURI S,MANDAL A,DEY A,et al.Tuning the swelling and rheological attributes of bentonite clay modified starch grafted polyacrylic acid based hydrogel[J].Applied Clay Science,2020,185:105405.

    23. [23]

      LIN F C,ZHENG J J,GUO W H,et al.Smart cellulose-derived magnetic hydrogel with rapid swelling and deswelling properties for remotely controlled drug release[J].Cellulose,2019,26(11):6861-6877.

    24. [24]

      EMAM H E,SHAHEEN T I.Design of a dual pH and temperature responsive hydrogel based on esterified cellulose nanocrystals for potential drug release[J].Carbohydrate Polymers,2022,278:118925.

    25. [25]

      BUENO V B,BENTINI R,CATALANI L H,et al.Synthesis and swelling behavior of xanthan-based hydrogels[J].Carbohydrate Polymers,2013,92(2):1091-1099.

    26. [26]

      GHOBASHY M M,ELBARBARY A M,HEGAZY D E.Gamma radiation synthesis of a novel amphiphilic terpolymer hydrogel pH-responsive based chitosan for colon cancer drug delivery[J].Carbohydrate Polymers,2021,263:117975.

    27. [27]

      DAI H J,CHEN Y,MA L,et al.Direct regeneration of hydrogels based on lemon peel and its isolated microcrystalline cellulose:Characterization and application for methylene blue adsorption[J].International Journal of Biological Macromolecules,2021,191:129-138.

    28. [28]

      DABROWSKI A.Adsorption-from theory to practice[J].Advances in Colloid and Interface Science,2001,93(1):135-224.

    29. [29]

      LANGMUIR I.The adsorption of gases on plane surfaces of glass,mica and platinum[J].Journal of the American Chemical Society,1918,40(9):1361-1403.

    30. [30]

      FREUNDLICH H.Over the adsorption in solution[J].Journal of Physical Chemistry,1906,57(4):385-470.

    31. [31]

      SAFAVI-MIRMAHALLEH S,SALAMI-KALAJAHI M,ROGHANI-MAMAQANI H.Effect of surface chemistry and content of nanocrystalline cellulose on removal of methylene blue from wastewater by poly (acrylic acid)/nanocrystalline cellulose nanocomposite hydrogels[J].Cellulose,2019,26(9):5603-5619.

    32. [32]

      CHEN X X,CHEN C,ZHU J.Facile preparation of cellulose-attapulgite nanocomposite hydrogel for dye adsorption[J].Iranian Polymer Journal,2019,28(4):347-359.

    33. [33]

      BEYRANVAND N S,SAMIEY B,TEHRANI A D,et al.Graphene oxide-cellulose nanowhisker hydrogel nanocomposite as a novel adsorbent for methylene blue[J].Journal of Chemical&Engineering Data,2019,64(12):5558-5570.

    1. [1]

      吴靖娜 , 林泽烨 , 苏筱 , 张任翔 , 陈晓婷 , 潘南 . 龙须菜渣纤维素/纳米纤维素及其水凝胶的制备和性能研究. 轻工学报, 2024, 39(6): 49-56. doi: 10.12187/2024.06.006

    2. [2]

      许克静 , 刘语煊 , 张展 , 吕晶晶 , 梁淼 , 李瑞丽 , 张峻松 , 陈小龙 . 辊压法全烟梗再造烟叶的制备工艺优化及结构与性能分析. 轻工学报, 2025, 40(1): 64-74. doi: 10.12187/2025.01.008

    3. [3]

      胡新楠 , 朱成凯 , 胡中泽 , 纪执立 , 金伟平 , 郭城 , 沈汪洋 . 复配比对明胶-羟丙基甲基纤维素双水相体系微观结构和流变特性的影响. 轻工学报, 2025, 40(1): 11-20. doi: 10.12187/2025.01.002

    4. [4]

      胡仙妹 , 于美逍 , 杨雪鹏 , 张展 , 尹献忠 . 木醋杆菌和酿酒酵母混菌发酵对烟用细菌纤维素品质的影响. 轻工学报, 2024, 39(6): 84-92. doi: 10.12187/2024.06.010

    5. [5]

      杨靖 , 刘广昊 , 王琼波 , 韩丽 , 王清福 , 赵志伟 , 李蕾 , 王秋领 . 微生物发酵开发杏果渣香料的研究. 轻工学报, 2024, 0(0): -.

    6. [6]

      兰玉婷 , 张逸飞 , 郭佳慧 , 尚欣欣 , 刘影 , 梁文魁 , 王璐 , 关国平 . 面向皮肤光电治疗术后热损伤护理的凝胶贴膜材料研究. 轻工学报, 2025, 40(1): 120-126. doi: 10.12187/2025.01.014

    7. [7]

      吕金羚 , 傅亮 , 陈永生 . 红茶-花生蛋白复合饮品工艺优化及其营养特性研究. 轻工学报, 2024, 0(0): -.

    8. [8]

      吕金羚 , 傅亮 , 陈永生 . 红茶-花生蛋白复合饮品工艺优化及其营养特性研究. 轻工学报, 2024, 39(5): 9-17. doi: 10.12187/2024.05.002

    9. [9]

      钟昕怡 , 陈紫麟 , 骆勇 , 汪高玮 , 王周利 , 赵子丹 , 李鸣雷 . 香菇-大球盖菇复合饼干研制及其品质特性分析. 轻工学报, 2024, 39(6): 27-36. doi: 10.12187/2024.06.004

    10. [10]

      曾强 , 阙文豪 , 许璧麟 , 于静 , 王昭焜 , 张尧立 , 张炜 , 董文亮 . 薄板烘丝机筒内结垢程度对设备工艺性能的影响. 轻工学报, 2025, 40(1): 58-63. doi: 10.12187/2025.01.007

    11. [11]

      楚文娟 , 郭丽霞 , 程东旭 , 王红霞 , 崔廷 , 冯银龙 , 王建民 , 鲁平 . 基于K-means聚类及模糊判别的卷烟包灰性能综合评价方法. 轻工学报, 2024, 39(6): 93-100. doi: 10.12187/2024.06.011

    12. [12]

      王春琼 , 刘凯 , 谢永辉 , 张轲 , 刘春明 , 张晓伟 , 孙浩巍 , 陈丹 . 烟草花叶病毒胶体金检测试纸条的制备与性能评价. 轻工学报, 2025, 40(1): 90-97. doi: 10.12187/2025.01.011

    13. [13]

      池哲翔 , 廖敏 , 史尚 , 李声毅 , 廖芸 , 丁冬 . 国外烟草活性成分提取及纤维材料利用现状与展望. 轻工学报, 2024, 0(0): -.

    14. [14]

      倪众 , 楚鹏飞 , 林颖 , 刘玉欣 . 低温长时间热处理过程中氧化和加热对海参体壁胶原纤维结构的影响. 轻工学报, 2025, 40(1): 21-31,57. doi: 10.12187/2025.01.003

  • 加载中
WeChat 点击查看大图
计量
  • PDF下载量:  23
  • 文章访问数:  2207
  • 引证文献数: 0
文章相关
  • 收稿日期:  2022-03-05
通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索
罗钰湲, 李辛娅, 梁佳翔, 等. 菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能[J]. 轻工学报, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
引用本文: 罗钰湲, 李辛娅, 梁佳翔, 等. 菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能[J]. 轻工学报, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
shu
LUO Yuyuan, LI Xinya, LIANG Jiaxiang, et al. Preparation and dye adsorption properties of pineapple peel cellulose/bentonite composite hydrogels[J]. Journal of Light Industry, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
Citation: LUO Yuyuan, LI Xinya, LIANG Jiaxiang, et al. Preparation and dye adsorption properties of pineapple peel cellulose/bentonite composite hydrogels[J]. Journal of Light Industry, 2022, 37(5): 41-49. doi: 10.12187/2022.05.005
shu

菠萝皮渣纤维素/皂土复合水凝胶的制备及其染料吸附性能

    作者简介:罗钰湲(1999-),女,重庆市人,西南大学硕士研究生,主要研究方向为纤维素及蛋白食品胶体。E-mail:854261043@qq.com
  • 1. 西南大学 食品科学学院, 重庆 400715;
  • 2. 重庆市朝阳中学, 重庆 400700
  • 收稿日期: 2022-03-05
基金项目:  重庆市雏鹰计划项目(CY210202)国家自然科学基金项目(31901683)重庆市自然科学基金项目(cstc2020jcyj-msxmX0087)

摘要: 以菠萝皮渣纤维素(PPC)为原料,通过碱/尿素体系溶解纤维素并掺入皂土,利用化学交联和原位嵌入磁性Fe3O4制备复合水凝胶,并对其结构和染料吸附性能进行研究。结果表明:皂土和Fe3O4在复合水凝胶中成功嵌入,皂土有效改善了水凝胶的交联多孔网络结构、热稳定性和溶胀性能。此外,添加皂土有利于提高水凝胶对亚甲基蓝的吸附性能,其饱和吸附量从28.09 mg/g提高到55.87 mg/g;吸附过程符合准二级动力学模型和Langmuir模型,属于化学吸附和单分子层吸附过程。

English Abstract

参考文献 (33) 相关文章 (14)

目录

/

返回文章

网站版权 © 轻工学报编辑部

地址：河南省郑州市科学大道136号邮编：450001

本系统由北京仁和汇智信息技术有限公司开发 技术支持： info@rhhz.net